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Does the Future Fantasy collection fit with, broadly speaking, the Modern City set? I want some more futuristic interiors for some buildings and this seems ideal but I can't quite tell whether it'll stand out too much. 

I'm not sure which set you mean. This Future Fantasy pack includes tiles for a modern city. Thanks!

Sorry, when I said Modern City, I meant your Omega Modern tileset.

Omega Modern is the same size, so it would be semi-compatible. The color is a different style though. Most objects from Omega Modern would fit fine if you edit the colors to match.